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After graduating from Silsbee High School in 1994, she became a model and pornographic actress. Jones was the Penthouse Pet of the Month in April 1998 and crossed over into adult films in 2001, then retired from the adult industry in 2004. She performed in eighteen films during this time. Jones had gained considerable fame as a nude model and was a well-known figure in the adult world at the time of her retirement.
Jones suffered multiple fractures to her arm in January 2000. She also reportedly suffered from epilepsy, however this is denied by her sisters as they claim that it was a move by her to gain attention.
Before Jones was able to make her comeback, however, her health began to fail. She died less than two weeks before her thirtieth birthday. The official cause was attributed to liver failure caused by years of alcohol and prescription drug abuse. She was addicted to the painkiller Vicodin. She would allegedly down 10 pills at a time and wash them down with Wild Turkey bourbon. In the end, Chloe Jones died in a charity hospital. She was buried at Woodlawn Garden of Memories in Houston, Texas.